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Data were collected on the 27th of November 2008 and on the 6th of January 2009 by the University of Manchester scanning mobility particle sizer at the Chilbolton site in support of the FAAM Campaign in the South-West of England. The dataset contains measurements of concentrations of aerosols of specific sizes. The data were collected for use in the ICE project, which is one of multiple projects within the APPRAISE (Aerosol Properties, PRocesses And Influences on the Earth's climate) programme.