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The Infrared Atmospheric Sounding Interferometer (IASI) methane dataset contains height-resolved and column-averaged volume mixing ratios of atmospheric methane (CH4). It also includes column-averaged water vapour (H2O), a scale factor for the HDO volume mixing ratio profile, surface temperature, effective cloud fraction, effective cloud-top pressure and scale factors for two systematic residual spectra which are jointly retrieved from the spectral range 1232.25-1290.00 cm-1 by the Rutherford Appleton Laboratory (RAL) IASI optimal estimation methane retrieval scheme. The dataset additionally contains selected a priori values and uncertainties adopted in the optimal estimation scheme and retrieval output diagnostics such as the retrieval cost and the averaging kernels. This work was funded by the National Centre for Earth Observation (NCEO) under the UK Natural Environment Research Council (NERC) with additional funding from EUMETSAT. Data were produced by the Science and Technology Facilities Council (STFC) Remote Sensing Group (RSG) at the Rutherford Appleton Laboratory (RAL). This is version 1.0 of this dataset and is the first to be released.